Fyzikální ústav Akademie věd ČR

Defect Engineering in Ce-Doped Aluminum Garnet Single Crystal Scintillators

M. Nikl1, K. Kamada2, V. Babin1, J. Pejchal1,2, K. Pilarova3, E. Mihokova1, A. Beitlerova1, K. Bartosiewicz1, S. Kurosawa2,4, A. Yoshikawa2,4

Mg-codoped Lu3Al5O12:Ce single crystal garnet scintillators were prepared with a wide concentration range 0–3000 ppm of Mg2+. Luminescence and scintillation characteristics were measured revealing the beneficial effect of Mg codoping which consists in stabilization of Ce4+ center. We propose a model explaining the mechanism of material improvement; the stable Ce4+ center provides an additional fast radiative recombination pathway in the scintillation mechanism.

Monocrystals prepared by "micropulling-down" method with marked level of Mg2+ additional dose.

1Institute of Physics AS CR, Cukrovarnicka 10, 16253 Prague, Czech Republic
2 New Industry Creation Hatchery Center (NICHe), Tohoku University, 6-6-10 Aoba, Aramaki, Aoba-ku, Sendai, Miyagi, Japan
3 Faculty of Nuclear Sciences and Physical Engineering, Czech Technical University in Prague, Brehova 7, 115 19 Prague, Czech Republic
4 Institute for Materials Research, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai, 980-8577 Japan

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